Quantum transport with electronic relaxation in electrodes: Landauer-type formulas derived from the driven Liouville–von Neumann approach

Abstract

We derive the exact steady-state solutions for the simplest model systems of resonant tunneling and tunneling with destructive quantum interference from the driven Liouville-von Neumann (DLvN) approach. Under the finite-state lead condition (the two electrodes have finite states), we analyze the asymptotic behavior of the steady-state current in the two limits of electronic relaxation. Under the infinite-state lead condition, the steady-state solutions of the two model systems can be cast as Landauer-type current formulas. According to the formulas, we show that the transmission functions near the resonant peak and the antiresonant dip can be significantly influenced by electronic relaxation in the electrodes. Moreover, under intermediate and strong electronic relaxation conditions, we analytically show that the steady-state current of the DLvN approach dramatically deviates from the Landauer current when destructive quantum interference occurs. In the regime of zero electronic relaxation, our results are reduced to the Landauer formula, indicating that the DLvN approach is equivalent to the Landauer approach when the leads have infinite states without any electronic relaxation.