Abstract

We have studied the electronic structure of electron-doped cuprate superconductors via measurements of high-field Shubnikov–de Haas oscillations in thin films. In optimally doped Pr2−xCexCuO4±δ and La2−xCexCuO4±δ, quantum oscillations indicate the presence of a small Fermi surface, demonstrating that electronic reconstruction is a general feature of the electron-doped cuprates, despite the location of the superconducting dome at very different doping levels. Negative high-field magnetoresistance is correlated with an anomalous low-temperature change in scattering that modifies the amplitude of quantum oscillations. This behavior is consistent with effects attributed to spin fluctuations.

Highlights

  • The fundamentals of the electronic interactions in the copper oxide family of superconductors remain a subject of intense debate

  • Pr2−xCexCuO4±δ and La2−xCexCuO4±δ, quantum oscillations indicate the presence of a small Fermi surface, demonstrating that electronic reconstruction is a general feature of the electron-doped cuprates, despite the location of the superconducting dome at very different doping levels

  • To understand how the choice of rare earth element affects the Fermi surface (FS), we report here measurements of quantum oscillations in thin films of PCCO for x < xc and x > xc and in optimally doped LCCO, which can only be stabilized in film form [22, 23]

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Summary

Introduction

The fundamentals of the electronic interactions in the copper oxide family of superconductors (cuprates) remain a subject of intense debate. One open question of particular importance is the nature of the normal state from which superconductivity emerges—whether it resembles a metal, having well-defined electron-like excitations, or a more exotic electronic phase. In hole-doped cuprates, the presence of a ‘pseudogap’ phase leads to even more uncertainty about the nature of the normal state. A schematic superconducting phase diagram for the electron-doped cuprates is shown in figure 1(a). The value of x for which the superconducting transition Tc is maximum is xo = 0.11 for La, 0.145 for Nd, and 0.15 for Pr. The actual cerium concentrations that determine the superconducting dome vary among the electron-doped cuprates, the general shape of the phase diagram is constant [6]

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