Abstract

Quantum oscillations measurements on PdCrO${}_{2}$ show that the Fermi surface of the antiferromagnetically ordered state is a consequence of reconstruction of the Fermi surface of the unordered state.

Highlights

  • We report quantum oscillation data on the metallic triangular antiferromagnet PdCrO2

  • To very high accuracy, the observed frequencies of PdCrO2 can be reproduced by reconstruction of the PdCoO2 Fermi surface int√o a re√duced zone

  • We present measurements of quantum oscillations in PdCrO2, and confirm the overall frequencies reported in Ref. [14]

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Summary

Introduction

We report quantum oscillation data on the metallic triangular antiferromagnet PdCrO2. A prominent example is the insulating CrO2 sheet, stabilized in materials such as LiCrO2 and PdCrO2. In these compounds, the Cr formal charge is +3, and its configuration is 3d3. Of materials containing such a CrO2 sheet, AgCrO2, CuCrO2, and PdCrO2 have the delafossite crystal structure, while LiCrO2, NaCrO2, and KCrO2 have the closely related ordered rock salt structure. The ordered rock-salt structure gives substantially smaller interplane spacings than the delafossite structure, and somewhat higher Neel temperatures [1]

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