Abstract
This work deals with the quantum-mechanical calculation of the temperature-dependent mobility of ionic lithium atoms diffusing in their parent gas. The computation of the quantal phase shifts in connection with the gerade and ungerade potential-energy curves, through which Li(+) approaches Li(2s), leads to the computation of the charge-transfer and diffusion cross sections. The behavior of the coefficients of diffusion and mobility with temperature is also examined. Throughout this work, the isotopic effects in the (6)Li(+)-(6)Li and (7)Li(+)-(6)Li collisions are emphasized.
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