Abstract
We present a scheme to control the generated ultrafast magnetic field in molecules using multi-frequency tricircular pulses composed of co- and counter-rotating bicircular pulses. Simulations show that the field amplitude and the wavelength are two significant factors for magnetic field generation by tricircular pulses. Specifically, the strength of the magnetic field is linearly related to the field amplitude at λ 0 = 50 nm, while at λ 0 = 70 nm, the strength first increases and then decreases with the amplitude, this can be attributed to the resonance between the ground and excited states. Moreover, the phase and helicity of bicircular pulses are shown to have important effects on the magnetic field. The dependence of the magnetic field on the phase arises from the interference effect between multiple ionization pathways. These findings illustrate a guiding principle for controlling the magnetic field in molecular systems for future research in ultrafast magneto-optics.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.