Abstract
The enhancement and tunable color emissions from codoped lanthanide ions of Er3+/Tm3+/Yb3+ have been studied extensively in recent decades. In this paper, we present a new scheme for quantum coherent control of two-photon absorption (TPA) and color emission in codoped lanthanide ions of Er3+/Tm3+/Yb3+ by properly phase shaping two infrared ultrashort laser beams at central frequencies of 10 650 cm−1 and 7650 cm−1, respectively. Compared with the results irradiated by transform-limited pulses, the TPA probabilities of the blue, green and red emissions are independently controlled in the ranges 0–13.3, 0–14.5 and 0–1.0, respectively. The effects of the energy states of lanthanide ions and the laser spectral bandwidths on the coherent features are also discussed. The TPA probabilities for the blue and green emissions increase with the laser spectral bandwidths and decrease with the energy bandwidths of the final level states. As the intermediate energy level shifts in the range 10 100–10 500 cm−1, the TPA probabilities for the blue and green emissions change in the ranges 7–15 and 8–17, respectively.
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