Abstract
We have applied conventional Time Differential Perturbed Angular Correlation (TDPAC) method to observe the anisotropy oscillations in the 3γ annihilation decay of polarized Positronium in a weak magnetic field. The effect, as predicted theoretically and experimentally demonstrated by Barishevsky et al. [V.G. Barishevsky, O.N. Metelitsa, V.V. Tikhomirov, Oscillations of the positronium decay γ-quantum angular distribution in a magnetic field, J. Phys. B: At. Mol. Opt. Phys.22 (1989) 2835], is induced by the coherent admixture of the m = 0 states of ortho-Positronium ( o-Ps) and para-Positronium ( p-Ps) in interaction with the magnetic field. The following experimental characteristics are to be considered: (i) the oscillation frequency corresponds to the difference in energy of the Ps atom levels in magnetic field and is proportional with H 2; (ii) in a fixed geometry the modulation depth (oscillations amplitude) depends on the mean positron polarization; (iii) privileged angles of the polarization vector, magnetic field and detectors are required for optimizing the observed oscillations amplitude. The normalized difference spectrum function ( R( t)) obtained from time spectra measured in vacuum and in different gaseous atmospheres (Ar, H 2, N 2) have the oscillations amplitude constant and we conclude that the Ps atoms are not fully thermalized over a time interval of about 400 ns. The R( t) functions obtained for o-Ps annihilation decays, in dry air or Ar–O mixture, have the oscillations amplitude time dependent due, probably, to the paramagnetism of the Oxygen molecules.
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