Abstract

We employ a recently developed quantization scheme for quasinormal modes (QNMs) to study a nonperturbative open cavity-QED system consisting of a hybrid metal-dielectric resonator coupled to a quantum emitter. This hybrid cavity system allows one to explore the complex coupling between a low $Q$ (quality factor) resonance and a high $Q$ resonance, manifesting in a striking Fano resonance, an effect that is not captured by traditional quantization schemes using normal modes or a Jaynes-Cummings (JC) type model. The QNM quantization approach rigorously includes dissipative coupling between the QNMs, and is supplemented with generalized input-output relations for the output electric field operator for multiple modes in the system, and correlation functions outside the system. The role of the dissipation-induced mode coupling is explored in the strong coupling regime between the photons and emitter beyond the first rung of the JC dressed-state ladder. Important differences in the quantum master equation and input-output relations between the QNM quantum model and phenomenological dissipative JC models are found. In a second step, numerical results for the Fock distributions and system as well as output correlation functions obtained from the quantized QNM model for the hybrid structure are compared with results from a phenomenological approach. We demonstrate explicitly how the quantized QNM model manifests in multiphoton quantum correlations beyond what is predicted by the usual JC models.

Highlights

  • Quantum emitters coupled to photons and/or plasmons in dissipative nanostructures, such as micropillars [1,2,3], photonic crystal cavities [4,5], dielectric microdiscs [6], or metallic nanoparticles [7,8,9,10,11], constitute an important field in quantum optics and quantum plasmonics

  • The two-level system (TLS) interacts with an effective semiclassical excitation field EL(ra, ω), which reflects a contribution of an incident laser field at the quantum emitter position, that is enhanced by the scattering structures in the dielectric medium, and a medium-assisted quantized electromagnetic field E, which obeys the quantized Helmholtz equation:

  • We briefly summarize the analysis in this subsection: For moderate pumping with respect to the PC mode, ∼ Gpc, the quasinormal modes (QNMs)-JC model exhibits a relatively high probability to be in a one- or two-excitation state for the PC-like mode (Ppc ≈ 0.4 and Ppc−pc ≈ 0.2), while the vacuum state |φvac is suppressed, when the laser is tuned in the regime of the PC-like cavity mode frequency

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Summary

INTRODUCTION

Quantum emitters coupled to photons and/or plasmons in dissipative nanostructures, such as micropillars [1,2,3], photonic crystal cavities [4,5], dielectric microdiscs [6], or metallic nanoparticles [7,8,9,10,11], constitute an important field in quantum optics and quantum plasmonics. While in the single-mode case, the results from a more phenomenological dissipative JC model is modified by a loss-induced prefactor, which separates between radiative and nonradiative decay [45], there are additional changes in the multimode case due to off-diagonal mode interaction, which influences the output coupling This may effect the behavior of multimode systems in higher rungs of the JC ladder, e.g., the change of Poissionian to sub-Possionian light when coupling a resonator-emitter system to another resonator, which is often described with two uncoupled modes [51,52]. We complement the main part of this work with six Appendixes that contain a more thorough derivation of the QNM input-output relations, further details of the QNM parameters of the hybrid structure, a detailed derivation of the photon correlation functions, as well as discussions about the light-matter coupling regimes of the hybrid structure, the response of the hybrid cavity to the external driving, and the treatment of the frequency integrals in the case of a few QNM expansion

Green’s function quantization approach
Quantized quasinormal mode approach
Multi-quasinormal-mode master equation
Diagonalization of the Lindblad dissipator
Input-output relations and output electric field operator
APPLICATIONS TO COUPLED OPEN RESONATORS
Weak light-exciton coupling regime
Strong light-exciton coupling
Eigenenergies and eigenstates
Steady-state probabilities and occupation numbers
Strong light-electron coupling
Output far field intensity
Second-order quantum correlation functions
Findings
CONCLUSIONS
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