Abstract
Abstract Quantitative analysis of line edge roughness (LER) is very important for understanding the root causes of LER and thereby improving the pattern quality in near-field lithography (NFL), because LER has become the main limiter of critical dimension (CD) control as the feature size of nanostructures is scaled down. To address this challenge, the photoresist point-spread function of NFL with a contact plasmonic ridge nanoaperture can be employed to account for the physical and chemical effects involved in the LER-generation mechanism. Our theoretical and experimental results show that the sources of LER in NFL mainly come from the aerial image, material chemistry, and process. Importantly, the complicated decay characteristics of surface plasmon waves are demonstrated to be the main optical contributor. Because the evanescent mode of surface plasmon polaritons (SPPs) and quasi-spherical waves (QSWs) decay in the lateral direction, they can induce a small image log-slope and low photoresist contrast, leading to a large LER. We introduce an analytical model and demonstrate the relationship between LER and CD to estimate the pattern quality in NFL. We expect that these results can provide alternative approaches to further improve pattern uniformity and resolution, which can lead to advanced nanopatterning results in NFL.
Highlights
We mainly discussed the physical concepts behind line edge roughness (LER) generation in near-field lithography (NFL), and predicted the generated LER quantitatively using an approximate analytical solution
A PR point-spread function (PSF), which was determined by the evanescent model of the quasi-spherical waves (QSWs) and surface plasmon polaritons (SPPs), was employed to quantitatively analyze the effect of the decay characteristics in the lateral direction on LER generation in NFL
We demonstrated that the rapid decay of the evanescent field can induce a large loss in the PR contrast, leading to a high LER
Summary
Near-field lithography (NFL) is a sub-diffraction-limited nanopatterning technology by exploiting surface plasmon polaritons (SPPs) and the diffracted field such as quasi-spherical waves (QSWs) [1,2,3,4,5,6,7,8,9,10,11,12,13,14,15,16,17,18,19,20]. We investigate the effect of the decay characteristics of evanescent waves on the ILS and PR contrast and further clarify the generation mechanism of LER in NFL using a plasmonic bowtie-shaped nanoaperture. The dominance of the evanescent field is further experimentally and theoretically investigated by increasing the ILS via control of the gap size These analyses are expected to provide useful guidance in minimizing the feature errors and effectively enhancing the pattern uniformity in the near-field nanopatterning process
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