Abstract

Ultraviolet (UV) SO2 cameras have become a common tool to measure and monitor SO2 emission rates, mostly from volcanoes but also from anthropogenic sources (e.g., power plants or ships). Over the past decade, the analysis of UV SO2 camera data has seen many improvements. As a result, for many of the required analysis steps, several alternatives exist today (e.g., cell vs. DOAS based camera calibration; optical flow vs. cross-correlation based gas-velocity retrieval). This inspired the development of Pyplis (Python plume imaging software), an open-source software toolbox written in Python 2.7, which unifies the most prevalent methods from literature within a single, cross-platform analysis framework. Pyplis comprises a vast collection of algorithms relevant for the analysis of UV SO2 camera data. These include several routines to retrieve plume background radiances as well as routines for cell and DOAS based camera calibration. The latter includes two independent methods to identify the DOAS field-of-view (FOV) within the camera images (based on (1) Pearson correlation and (2) IFR inversion method). Plume velocities can be retrieved using an optical flow algorithm as well as signal cross-correlation. Furthermore, Pyplis includes a routine to perform a first order correction of the signal dilution effect (also referred to as light dilution). All required geometrical calculations are performed within a 3D model environment allowing for distance retrievals to plume and local terrain features on a pixel basis. SO2 emission rates can be retrieved simultaneously for an arbitrary number of plume intersections. Hence, Pyplis provides a state-of-the-art framework for more efficient and flexible analyses of UV SO2 camera data and, therefore, marks an important step forward towards more transparency, reliability and inter-comparability of the results. Pyplis has been extensively and successfully tested using data from several field campaigns. Here, the main features are introduced using a dataset obtained at Mt. Etna, Italy on 16 September 2015.

Highlights

  • Sulfur dioxide (SO2 ) is a toxic gas emitted by anthropogenic and natural sources

  • Prominent examples for passive remote sensing instrumentation are the correlation spectrometer (COSPEC, [7]), or instruments based on the technique of Differential Optical Absorption Spectroscopy (DOAS, [8], e.g., [9,10])

  • The DOAS calibration is performed using a set of plume optical density images and a corresponding time-series of SO2 -CDs retrieved from a DOAS spectrometer

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Summary

Introduction

Sulfur dioxide (SO2 ) is a toxic gas emitted by anthropogenic and natural sources (e.g., power plants, ships, volcanoes). The comparatively young technique of UV SO2 cameras has gained in importance, since it enables the study of volcanic SO2 emissions at unprecedented spatial and temporal resolution (e.g., [11,12,13,14,15]) This is helpful to study multiple sources independently (e.g., [16]) or to investigate volcanic degassing characteristics by studying periodicities in the SO2 emission rates (e.g., [17,18,19] and references therein).

UV SO2 Cameras
Image Analysis—Retrieval of SSO2 Images
Emission Rate Retrieval
Radiative Transfer Corrections
Implementation
Geometrical Calculations
Image Representation and Pre-Processing Routines
Retrieval of Plume Background Radiances
Method
Calibration Using SO2 Cells
Calibration Using DOAS Data
DOAS FOV Search
Plume Velocity Analysis
Velocity Retrieval Using the ICA Cross-Correlation Method
Optical Flow Based Velocity Retrievals
Image Based Signal Dilution Correction
Remark on Uncertainties
Conclusions
Introduction into ImgList objects
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