Abstract
Pulsed electron-electron double resonance techniques have been applied to the \ifmmode \dot{C}\else \.{C}\fi{}H fragment in an irradiated single crystal of malonic acid. Damped Torrey oscillations about the pumping field and also about the observing field have been observed, and the spin-lattice and cross-relaxation times have been measured directly. Display of the transient signal intensity at a constant delay as a function of the pump frequency (i.e., relaxation spectroscopy) yielded very narrow EPR hyperfine lines.
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