Abstract
Dunn and colleagues design and synthesize a thin film pseudo-solid state electrolyte for next-generation lithium batteries based on solution-processed ionogels. They first demonstrate 125 mAh/g capacity for 150 cycles with minimal capacity loss in lithium iron phosphate and lithium metal full cell devices at C/2 rate. Next, they demonstrate the ability to photo-pattern the ionogel, and thus enable versatile and scalable fabrication and processing routes, while also retaining similar excellent electrochemical performance.
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