Abstract
The quasi-free benzene rotation of paramagnetic V(C 6H 6) 2 substituted into Fe(C 5H 5) 2 and Cr(C 6H 6) 2 hosts has been studied by ENDOR spectroscopy between T = 15 K and T = 180 K. In Fe(C 5H 5) 2, two different coalescence temperatures have been found. The full proton hfs tensor of the rigid molecule has been determined from powder samples.
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