Abstract

The spontaneous fission of $^{252}\mathrm{Cf}$ serves as an excellent benchmark of prompt emission in fission since experimental data can be obtained without the need of an incident beam. With the purpose of providing experimental data on the prompt fission neutron properties in correlation with fission-fragment characteristics, an experiment on $^{252}\mathrm{Cf}$(SF) has been performed. In addition, the experiment serves as a benchmark of setup and analysis procedures for measurements of fluctuations in the prompt-neutron properties as a function of incident neutron energy in fission of the major actinides $^{235}\mathrm{U}$ and $^{239}\mathrm{Pu}$. The experiment employs a twin Frisch grid ionization chamber as fission-fragment detector while neutrons were counted by using a liquid scintillator placed along the symmetry axis of the ionization chamber. Average neutron multiplicity has been obtained as a function of fission-fragment mass and total kinetic energy (TKE). The average multiplicity as a function of mass agrees well with available data in the literature in the mass range from 80 to 170 u. The existence of additional sawtooth structures in the far asymmetric mass region could not be confirmed, although the statistical accuracy of the present experiment is as good as the previous study where such structures have been reported [Nucl. Phys. A 490, 307 (1988).]. The available data in the literature on the TKE dependence of the multiplicity show strong deviations. Therefore, effort was focused on investigating experimental factors in low-efficiency neutron-counting experiments that may lead to faulty determination of this dependence. Taking these factors into account, a result that agrees well with data from high-efficiency neutron-counting experiments is obtained. The experimental arrangement allows determination of the angle between the detected neutron and the fission axis, which permits the neutron properties to be transformed into the fission-fragment rest frame. Fission neutron emission spectra in the fragment center-of-mass frame have thereby been obtained as a function of the fission-fragment mass and TKE.

Highlights

  • Investigation of prompt-fission neutron emission in fission is of particular importance in understanding the fission process

  • For nuclear modeling and improved evaluation of nuclear data, the knowledge of fluctuations in the promptneutron multiplicity as a function of incident neutron energy is requested for the major actinides 235U and 239Pu

  • Fluctuations in fission-fragment mass and total kinetic energy (TKE) in both isotopes have been observed in resonance neutron-induced fission [1,2]

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Summary

Introduction

Investigation of prompt-fission neutron emission in fission is of particular importance in understanding the fission process. Knowledge of the properties of prompt-fission neutrons, their multiplicities, and energy distributions could give answers to questions related to neutron emission itself and to questions relevant to the formation of the fission fragments, the sharing of excitation energy among them, and the timescale of the process. Fluctuations in the number of emitted neutrons have been observed [3]. In view of the fact that both neutron number and fission-fragment properties have been found to vary, it is necessary to understand to what extent the prompt neutron multiplicity is changing or if the observed fluctuations are due to the changes in the fission-fragment properties.

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