Abstract

In this paper we present new results for prompt fission $\ensuremath{\gamma}$-ray spectral characteristics from the thermal neutron induced fission of $^{240}\mathrm{Pu}^{*}$. The measured spectra were unfolded by using the detectors' response functions, simulated with geant4. We obtained in average per fission a $\ensuremath{\gamma}$-ray multiplicity ${\overline{M}}_{\ensuremath{\gamma}}=(7.35\ifmmode\pm\else\textpm\fi{}0.12)$, a mean photon energy ${\overline{\ensuremath{\epsilon}}}_{\ensuremath{\gamma}}=(0.85\ifmmode\pm\else\textpm\fi{}0.02)$ MeV, and an average total energy released in fission ${\overline{E}}_{\ensuremath{\gamma},\mathrm{tot}}=(6.27\ifmmode\pm\else\textpm\fi{}0.11)$ MeV. Our results are in good agreement with historical data measured in the 1970s by Verbinski et al. and results from recent calculations in the framework of Monte Carlo Hauser--Feshbach models. Our measured average total energy is slightly smaller than the one deduced previously and present in evaluated data. From this we conclude that the $^{239}\mathrm{Pu}({n}_{\mathrm{th}},f)$ reaction may be ruled out as possible source of $\ensuremath{\gamma}$ heating underestimation, when compared with benchmark calculations based on existing nuclear data.

Highlights

  • Recent benchmark exercises on nuclear reactors have revealed an underestimation of prompt γ heating by 10% to 28% for 235U and 239Pu [1]

  • Our results are in good agreement with historical data measured in the 1970s by Verbinski et al and results from recent calculations in the framework of Monte Carlo Hauser–Feshbach models

  • This has motivated a revival for measurements of prompt-fission γ -ray spectral (PFGS) characteristics, and international efforts have been put into improving the accuracy of data since the latest results dated from the 1970s

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Summary

INTRODUCTION

Recent benchmark exercises on nuclear reactors have revealed an underestimation of prompt γ heating by 10% to 28% for 235U and 239Pu [1]. This has motivated a revival for measurements of prompt-fission γ -ray spectral (PFGS) characteristics, and international efforts have been put into improving the accuracy of data since the latest results dated from the 1970s. The reaction 239Pu(n,f ) is the second of the two candidates on the High Priority Request List (HPRL) published by the OECD/NEA, beside 235U(nth,f ) [4], aiming to improve the precision of PFGS characteristics to an uncertainty lower than 7.5% [1]. A big challenge in the 239Pu(nth,f ) reaction measurement is the high specific alpha activity of 2 MBq/mg. Our results will be shown and compared with existing experimental data and model calculations

EXPERIMENTAL SETUP AND DATA ANALYSIS
Alpha and pileup rejection
Time-of-flight discrimination
The unfolded spectra
Evaluation
Average spectral characteristics
CONCLUSIONS
Methods
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