Abstract

Production cross sections of astatine isotopes 207−211At in the 29–57 MeV 7Li + natPb reaction have been measured by α- and γ-ray spectrometry. Excitation functions of production cross sections have been compared with a statistical calculation to study the reaction mechanism of the 7Li + natPb reaction. Production reactions of 207−211At in the 7Li + natPb have been derived. Considerably small experimental cross sections of 210At and 209At compared with the statistical calculation were clearly observed at incident energies higher than 44 MeV, indicating that the effects of breakup reaction play a role. A chemical separation of astatine from an irradiated lead target has been studied with a dry-distillation method. A complementary way to produce astatine isotopes has been developed.

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