Probing magnetic anisotropy and spin-reorientation transition in the three-dimensional antiferromagnet Ho0.5Dy0.5FeO3|Pt using spin Hall magnetoresistance

Abstract

Orthoferrites ($RE$FeO$_{3}$) containing rare-earth ($RE$) elements are 3D antiferromagnets (AFM) that exhibit characteristic weak ferromagnetism originating due to slight canting of the spin moments and display a rich variety of spin reorientation transitions in the magnetic field ($H$)-temperature ($T$) parameter space. We present spin Hall magnetoresistance (SMR) studies on a $b$-plate ($ac$-plane) of crystalline Ho$_{0.5}$Dy$_{0.5}$FeO$_{3}|$Pt (HDFO$|$Pt) hybrid at various $T$ in the range, 11 to 300 K. In the room temperature $\Gamma_4(G_x, A_y, F_z)$ phase, the switching between two degenerate domains, $\Gamma_4(+G_x, +F_z)$ and $\Gamma_4(-G_x, -F_z)$ occurs at fields above a critical value, $H_{\text{c}} \approx 713$ Oe. Under $H > H_{\text{c}}$, the angular dependence of SMR ($\alpha$-scan) in the $\Gamma_4(G_x, A_y, F_z)$ phase yielded a highly skewed curve with a sharp change (sign-reversal) along with a rotational hysteresis around $a$-axis. This hysteresis decreases with an increase in $H$. Notably, at $H < H_{\text{c}} $, the $\alpha$-scan measurements on the single domain, $\Gamma_4(\pm G_x, \pm F_z)$ exhibited an anomalous sinusoidal signal of periodicity 360 deg. Low-$T$ SMR curves ($H$ = 2.4 kOe), showed a systematic narrowing of the hysteresis (down to 150 K) and a gradual reduction in the skewness (150 to 52 K), suggesting weakening of the anisotropy possibly due to the $T$-evolution of Fe-$RE$ exchange coupling. Below 25 K, the SMR modulation showed an abrupt change around the $c$-axis, marking the presence of $\Gamma_2(F_x,C_y,G_z)$ phase. We have employed a simple Hamiltonian and computed SMR to examine the observed skewed SMR modulation. In summary, SMR is found to be an effective tool to probe magnetic anisotropy as well as a spin reorientation in HDFO. Our spin-transport study highlights the potential of HDFO for future AFM spintronic devices.