Abstract

We report magnetization properties of (CuZr)93−xAl7Gdx bulk metallic glasses from temperature dependent 27Al nuclear magnetic resonance spectroscopy and magnetic susceptibility measurements. Significant non-linear line broadening of 27Al spectra commencing at high temperatures is attributed to the development of a local magnetic susceptibility distribution that prevails over a finite temperature range. Magnetization measurements confirm the linewidth enhancement due to strong frustrated magnetic short-range order. This study provides insight into the nature of magnetic development and frustration in paramagnetic systems.

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