Probing Evolution of the Flux-Pinning Landscape in REBCO Coated Conductors Caused by Gamma Irradiation Using DC and AC Magnetometry: A Novel Approach to Tokamak Magnet Material Development

Abstract

Optimisation of REBCO coated conductor tapes specifically for use in nuclear fusion will help improve the magnet component lifetimes in future tokamak reactor power plants. The focus of this work was exploration of a novel approach to irradiation studies on REBCO tapes, utilising multiple magnetic measurements to probe evolution of the REBCO flux-pinning landscape more deeply than reported in other studies, for the purpose of identifying primary limiting factors affecting performance. Gamma irradiation experiments were conducted, and pre-/post-irradiation results from DC and AC magnetic measurements using a Physical Property Measurement System (PPMS) are discussed. Magnetisation critical current density (Jc) decreased in all samples with increasing dose, except for the silver overlayer-only samples which did not contain artificial pinning centres (APCs), where Jc increased with dose. Removal of the copper stabiliser coupled with the presence of APCs allowed gamma irradiation to induce pinning force maximum peak shifts, from above 14 T before irradiation to below 9 T afterwards. Flux creep rate varied with the evolving pinning landscape, and the degree of Jc degradation directly correlated with creep rate fluctuations post-irradiation. Changes in critical temperature and diamagnetic saturation also corresponded with changes in Jc and flux creep rate. The major conclusion from this study was that minimisation of flux creep rate is the key to maintenance of performance under fusion-relevant operating conditions. Flux creep manifests as problematic AC losses in all high-temperature superconducting machines; therefore, future work will focus on reduction/prevention of the phenomenon to enhance longevity of performance in any application.