Primary ice nucleation in orographic cirrus clouds: A numerical simulation of the microphysics

Abstract

AbstractIce particle production by the processes of homogeneous freezing and heterogeneous nucleation in orographic cirrus clouds is studied using a simple adiabatic ascending‐air‐parcel model. Homogeneous freezing rates in the model are based on a formulation by Jeffery and Austin, which matches with observed rates, modified according to the solution effect. Two alternative ice nuclei (IN) activation spectra are applied, one dependent upon temperature and the other upon ice supersaturation. Simulations are performed for air parcels with initial dew‐point temperatures, Td, in the range from −20 to −45°C and constant vertical velocities, w, of 0.1 to 5.0 m s‐1. In modelled clouds with Td ⩾ 30°C, heterogeneous nucleation initiated by IN is found to dominate ice formation, since homogeneous freezing rates are so low. In modelled clouds with Td ⩽ −35°C, pure liquidwater homogeneous freezing rates are large, but inclusion of sufficient quantities of IN may completely suppress aqueous solution droplet growth, dilution and homogeneous freezing, with heterogeneous nucleation then remaining dominant even at very low temperatures. the IN number concentrations required for homogeneous freezing suppression, for a fixed cloud condensation nucleus (CCN) activation spectrum, are found to increase with increasing w‐heterogeneous nucleation at low temperatures is therefore much more viable at the low w values found in non‐orographic compared with orographic cirrus clouds. the common conception of a deficit of IN aloft is challenged, and, because of the apparent sensitivity of cirrus cloud microphysical and radiative properties to these aerosol particles, IN measurements at cirrus levels, in addition to CCN measurements, are suggested as vital. the model results suggest that it may be possible to interpret measurements of peak liquid‐water content, or possibly maximum droplet radius, in orographic cirrus clouds in terms of the dominant ice nucleation mode.