Abstract
Large enhancement of antiferromagnetic (AF) transition temperature T N by pressure was observed in a quasi two-dimensional organic conductor, β'-(Me 4 P)[Pd(dmit) 2 ] 2 . Similar results are obtained in Et2Me2P salt at 5 kbar. It is indicated that pressure tends to reduce magnetic frustrations leading to the stabilization on AF state. A single crystal of β'-(Et2Me2P)[Pd(dmit) 2 ] 2 was also examined at ambient pressure. A clear evidence of AF transition was obtained at around 16 K by 13 C NMR relaxation rate 1/T 1 . This is consistent with ESR study, but different from our polycrystalline experiments.
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