Abstract
A novel bis(imino nitroxide)-substituted resorcinol 3H, that has two metal-binding sites with two pairs of the phenolate anion and the imino nitrogen atom, was prepared. The powdered sample of 3H showed an intramolecular ferromagnetic interaction ( J/ k B = +5 K) between two (imino nitroxide)s through a m-phenylene bridge and a weak intermolecular antiferromagnetic interaction ( J/ k B = − 0.9 K). The reaction of 3H with copper acetate in methanolic ammonia was examined to give a hardly soluble Cu-complex that exhibited ferromagnetic behavior in relatively high temperatures (298–55 K).
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