Prediction of high-temperature infrared radiative properties of nickel foam ligaments

Abstract

High-temperature radiative properties of open-cell foam ligaments are rather sparse due to measurement limitation. This study aims to numerically predict the infrared radiative properties of nickel foam ligaments at high temperatures. In this work, rough surfaces of ligaments are modeled with SEM scanning pictures, and optical properties of nickel components are simulated using ab initio molecular dynamics method at 298 K, 673 K, 873 K, 1073 K and 1273 K. The reflectivity of smooth surface is determined with empirical formulas at high temperatures. Moreover, the spectral radiative properties of nickel foam ligaments are predicted with finite difference time domain method at the waveband of 0.8–8.5 μm based on the modeled surfaces and high-temperature optical properties of components. It is found high temperature can marginally strengthen radiation scattering of the ligament surfaces, while having little effect on the distribution of radiation scattering. For instance, the directional-hemispherical reflectivity increases approximately linearly with temperature. As the incident wavelength grows, the directional-hemispherical reflectivity and proportion of specular reflection both show a rapid increase in the studied waveband, while the value of reflection main peak of directional-hemispherical reflectivity declines. With the growth of incident angle, the center position of main reflection peak is moving to the direction of increasing angles. Polynomial fit is applied to anticipate the relationship between proportion of specular reflection and incident wavelength with a RSME less than 0.02. This work demonstrates a practical method for obtaining the infrared radiative properties of open-cell metal foam ligaments at high temperatures.