Abstract
Power plant plume measurements with instrumented aircraft indicate that the plume-environment reactant species (NO and O3) appear to be spatially segregated with reactions occurring primarily within a relatively narrow zone between the plume core and the environment. Within this reaction zone, the NO2/NO ratios reach a maximum and increase with plume travel time. Inhomogeneous mixing in the reaction zone appears to provide net ositive correlationg of the photostationary equilibrium (E) fluctuation term [NO]′[O3]′, which results in E ≫ 1 within the first hour of plume travel time.
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