Abstract
We report the synthesis and electron donor-acceptor features of a novel nanohybrid, in which the light-harvesting and electron-donating properties of a meso-tetraarylporphyrin (TArP) are combined with the electron-accepting features of nitrogen-doped carbon nanodots (NCNDs). In particular, in an ultrafast process (>1012 s-1 ), visible-light excitation transforms the strongly quenched porphyrin singlet excited states into short-lived (225 ps) charge-separated states. On the other hand, ultraviolet light excitation triggers a non-resolvable transduction of singlet excited state energy from the NCNDs to the porphyrins, followed by the same charge separation observed upon visible light excitation.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.