Abstract

Fracture experiments on polymer gels are often conducted with thin specimens, which are close to plane stress in two-dimensional models. However, many of the previous theoretical and numerical studies on fracture of polymer gels have assumed plane strain conditions. The subtle differences between the plane stress and plane strain conditions are elucidated in this paper based on a linear poroelastic formulation for polymer gels, including the asymptotic crack-tip fields and finite element simulations of steady-state crack growth in long strip specimens. Moreover, a poroelastic cohesive zone model is adopted to study the rate-dependent fracture process of polymer gels. It is found that, without the cohesive zone model, the normalized crack-tip energy release rate at the fast crack limit is greater than the slow crack limit, suggesting reduced poroelastic toughening for fast crack growth under plane stress conditions, while the two limits are identical under plane strain conditions. With a solvent-permeable cohesive zone for the case of immersed specimens, solvent diffusion within the cohesive zone enhances the poroelastic toughening significantly as the crack speed increases, leading to a rate-dependent traction-separation relation. On the other hand, with no solvent diffusion in the cohesive zone for the not-immersed case, the poroelastic toughening effect diminishes as the crack speed increases. Based on the present study, the intrinsic steady-state fracture toughness of a poroelastic gel can be determined using long-strip pure-shear specimens, which in general is smaller than the applied energy release rate.

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