Abstract

Surface PM2.5 concentrations are required for exposure assessment studies. Remotely sensed Aerosol Optical Depth (AOD) has been used to derive PM2.5 where ground data is unavailable. However, two key challenges in estimating surface PM2.5 from AOD using statistical models are (i) Satellite data gaps, and (ii) spatio-temporal variability in AOD-PM2.5 relationships. In this study, we estimated spatially continuous (0.03° × 0.03°) daily surface PM2.5 concentrations using MAIAC AOD over Madhya Pradesh (MP), central India for 2018 and 2019, and validated our results against surface measurements. Daily MAIAC AOD gaps were filled using MERRA-2 AOD. Imputed AOD together with MERRA-2 meteorology and land use information were then used to develop a linear mixed effect (LME) model. Finally, a geographically weighted regression was developed using the LME output to capture spatial variability in AOD-PM2.5 relationship. Final Cross-Validation (CV) correlation coefficient, r2, between modelled and observed PM2.5 varied from 0.359 to 0.689 while the Root Mean Squared Error (RMSE) varied from 15.83 to 35.85 µg m−3, over the entire study region during the study period. Strong seasonality was observed with winter seasons (2018 and 2019) PM2.5 concentration (mean value 82.54 µg m−3) being the highest and monsoon seasons being the lowest (mean value of 32.10 µg m−3). Our results show that MP had a mean PM2.5 concentration of 58.19 µg m−3 and 56.32 µg m−3 for 2018 and 2019, respectively, which likely caused total premature deaths of 0.106 million (0.086, 0.128) at the 95% confidence interval including 0.056 million (0.045, 0.067) deaths due to Ischemic Heart Disease (IHD), 0.037 million (0.031, 0.045) due to strokes, 0.012 million (0.009, 0.014) due to Chronic Obstructive Pulmonary Disease (COPD), and 1.2 thousand (1.0, 1.5) due to lung cancer (LNC) during this period.

Highlights

  • Increased cardiovascular and respiratory diseases in addition to a decreased life expectancy are associated with chronic exposure to particulate matter with aerodynamic diameters < 2.5 μm, ­PM2.51

  • Percentage frequency distribution of Aerosol Optical Depth (AOD), P­ M2.5, and meteorological variables used in the statistical models are summarized in Supplemental Figure S13

  • MERRA-2 AOD consistently underestimated the AOD over Madhya Pradesh compared to Multi-Angle Implementation of Atmospheric Correction (MAIAC) AOD

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Summary

Introduction

Increased cardiovascular and respiratory diseases in addition to a decreased life expectancy are associated with chronic exposure to particulate matter with aerodynamic diameters < 2.5 μm, ­PM2.51. A number of statistical models were developed to capture the varying relationships between AOD and surface P­ M2.5 concentrations at various locations across the world, such as the linear mixed effect model, geographically weighted regression, and generalized additive m­ odels[12,13]. These studies have used meteorological parameters (height of planetary boundary layer, surface temperature, wind speed, relative humidity) and land use information as covariates along with satellite AOD to estimate surface P­ M2.5 concentrations. An additional objective of this study was to utilize the derived concentrations to estimate the population exposure to P­ M2.5 and the associated premature mortality over Madhya Pradesh during 2018–2019

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