Abstract
The surfaces of materials fabricated from stainless steel are challenging to functionalize with antimicrobial moieties. This work demonstrates that stainless steel surfaces can be modified with an N-halamine-based copolymer in order to obtain antimicrobial activity. In this regard, a copolymer (HACM) of 2-acrylamido-2-methyl-1-(5-methylhydantoinyl)propane and 3-cloro-2-hydroxypropyl methacrylate was synthesized and grafted onto a stainless steel surface via covalent attachment. Synthesized monomers and copolymers were characterized by NMR, FTIR, and XPS spectral analyses. Upon treatment with dilute bleach, the stainless steel surfaces were rendered antimicrobial, possessing a sufficient amount of chlorine content and excellent stability and durability. The modified stainless steel samples inactivated 6 logs of Staphylococcus aureus and Escherichia coli O157:H7 bacteria within 15 min of contact time. Stabilities of the coatings toward washing and UVA exposure were also studied. The stainless steel samples ...
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