Abstract
Polarized IR and Raman spectra of the oriented benzophenone (C13H10O) crystal have been measured and discussed together with the LO-TO splitting of the polar modes. The normal modes are defined and assignment of the vibrational modes is proposed on the basis of quantum chemical calculations. The B3LYP/6-31G(d,p) quantum model and PED contributions have been applied in the discussion of the results. The obtained results have also been used for analysis of promoting modes in the stimulated Raman scattering effect. Copyright © 2005 John Wiley & Sons, Ltd.
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