Polarization Control in Three-Dimensional Resonant Coherent Excitation

Abstract

We present an experimental demonstration of an ingenious technique to control the alignment of the atomic internal state in the x-ray region using a periodic crystal field. The alignment directions of Ar16+ and Fe24+ ions were readily controlled by selecting the array of atomic planes using three-dimensional resonant coherent excitation, and were probed via the anisotropy of the deexcitation x-ray emission. We applied this method to a double resonance experiment, and succeeded in controlling the population of the specific magnetic substate in a Lambda-type three-level configuration.