Abstract

Measurements of the Rayleigh depolarization ratios (with and without inclusion of the vibrational Raman contributions), Cotton-Mouton effects and electric field-gradient induced birefringences of gaseous HCCH, HCCCH 3 and CH 3CCCH 3 at 632.8 nm are analyzed in conjunction with other data to obtain reliable values of the polarizability anisotropies, magnetizability anisotropies and quadrupole moments of these molecules.

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