Plasmonic nanoresonator distributions for uniform energy deposition in active targets

Abstract

Active targets implanted with core-shell-composition (CS) and nanorod-shaped (NR) plasmonic nanoresonators and doped with dyes were designed to ensure uniform energy deposition during illumination by two-counter propagating short laser pulses. The near-field enhancement, optical responses, and cross-sections were mapped above the concentration-Epump parameter-plane to inspect two different regions (I and II) with the potential to improve light-matter interaction phenomena. The distribution of steady-state absorption, as well as of the power-loss and power-loss density integrated until the complete overlap of the two short pulses was determined. The uniform distribution was adjusted to constrain standard deviations of the integrated power-loss distributions in the order of ∼10%. Dye doping of target-I/II implanted with uniform CS (NR) nanoresonator distributions results in larger absorption with increased standard deviation, larger power-loss, and power-loss density with decreased (decreased / increased) standard deviation. The adjustment allows larger absorption in CS-II and larger power-loss and power-loss density in CS-implanted targets, smaller standard deviation in targets-I for absorption, and in all targets for power-loss and its density. Larger dye concentration makes it possible to achieve larger absorption (except in adjusted NR-II), larger power-loss and power-loss density in all CS and in adjusted NR distributions, with decreased standard deviation in CS-implanted targets for all quantities and in NR-implanted targets for absorption. CS implantation results in larger absorption with a larger standard deviation, moreover allows larger power-loss in adjusted distributions and smaller standard deviation in power-loss quantities for larger concentration in both distributions and the same standard deviation for smaller concentration in adjusted distribution. Based on these results, adjusted CS distributions in targets doped with a dye of higher concentration are proposed.