Abstract

The aim of this work is to evaluate the influence of absorption processes on the Time Of Flight (TOF) of the light scattered out of a thick medium in the forward direction. We use a Monte-Carlo simulation with temporal phase function and Debye modes. The main result of our study is that absorption inside the particle induces a decrease of the TOF on a picosecond time scale, measurable with a femtosecond laser apparatus. This decrease, which exhibits a neat sensitivity to the absorption coefficient of particles, could provide an efficient way to measure this absorption.

Highlights

  • The understanding of interactions between light and scattering dense media such as clouds, paints or biological tissues is a major issue as far as optical diagnosis is concerned

  • The aim of this work is to evaluate the influence of absorption processes on the Time Of Flight (TOF) of the light scattered out of a thick medium in the forward direction

  • The main result of our study is that absorption inside the particle induces a decrease of the TOF on a picosecond time scale, measurable with a femtosecond laser apparatus

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Summary

Introduction

The understanding of interactions between light and scattering dense media such as clouds, paints or biological tissues is a major issue as far as optical diagnosis is concerned. Thanks to Optical Kerr Gate (OKG) measurements [8] or up-conversion technique [9], it is possible to temporally sample the light going out of the sample with a resolution of approximately 100 fs [10] (i.e. less than 20 microns spatially). Such experiments are used to isolate ballistic and scattered light (ballistic imaging [11, 12], optical density measurement [13]) or to study the temporal scattering process itself in order to get information about the sample [14,15,16]. This effect appears to be very sensitive to the imaginary part of the particle refractive index

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