Abstract
One of the basic questions in chemistry today is concerned with the degradation of energy in a molecular system. The time-dependent redistribution of energy among the various degrees of freedom within a molecule on excitation to some excited state and the interactions and energy exchange of the excited molecule with surrounding molecules and external fields are of fundamental importance to a description of molecular phenomena. It is the competition between the various dissipative pathways which determines whether light is emitted or nonradiative physical and chemical processes dominate in the degradation of energy and materials in the system of interest.
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