Abstract
Abstract We report a picosecond pump-probe study of the UV photolysis of gaseous dimethylnitramine. After photolysis by picosecond laser pulses at 266 nm, efficient monophotonic collision-free photodissociation occurs within 6 ps. NO 2 fragments are formed in the ground electronic state and in a fluorescent excited state; the quantum yields for both of these channels are estimated.
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