Abstract
The experimental results of time-resolved coherent resonance Stokes and anti-Stokes Raman scattering spectroscopy of the excited electronic S 1 state of trans-stilbene in ethanol are presented. The detected considerable changes in vibrational spectra due to “optical depiction” of the population of the S 1 state reflect the picosecond kinetics of vibrational-translational relaxation of vibrationally “hot” excited molecules.
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