Abstract
Molecular light-switch: Off–on switching of the fluorescence of the protein asFP595 involves a trans–cis isomerization. Mixed quantum/classical simulations elucidate the spectroscopic properties of asFP595 and give detailed insights into the photoswitching mechanism. The conformational trans–cis switching triggers a proton-transfer cascade between the chromophore and adjacent amino acids. Supporting information for this article is available on the WWW under http://www.wiley-vch.de/contents/jc_2002/2007/z602315_s.pdf or from the author. Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.
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