Abstract
Abstract The photolysis of (prophos)CuI(CO3)CuI(prophos) with prophos = 1,3-bis(diphenylphosphino)-propane in homogeneous solution leads to the reduction of carbonate according to a simple overall stoichiometry (CO2 + prophos → CO + prophos monoxide). It is suggested that this reaction is initiated by a ( Cu I → CO 3 2 - ) MLCT state.
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