Abstract
KrF excimer laser-induced reactions in the mixture of ethylene/O 2/CO 2 under sub- and super-critical conditions were investigated. The main products were acetaldehyde and ethylene oxide. The total quantum yield decreased with the increase of mixture density, but the branching ratio between the two products were almost independent on the density. The branching ratio was found to be what is expected if the reactive species is O( 3P). Any distinctive specific pressure effect has not been observed in the near-critical region.
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