Abstract

The conversion and interaction between quantum signals at the single-photon level are essential for scalable quantum photonic information technology. Using a fully optimized periodically poled lithium niobate microring, we demonstrate ultraefficient sum-frequency generation on a chip. The external quantum efficiency reaches $(65\ifmmode\pm\else\textpm\fi{}3)\mathrm{%}$ with only $(104\ifmmode\pm\else\textpm\fi{}4)$-$\ensuremath{\mu}\mathrm{W}$ pump power. At peak conversion, $3\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}5}$-noise photon is created during the cavity lifetime, which meets the requirement of quantum applications using single-photon pulses. Using a pump and signal in single-photon coherent states, we directly measure the conversion probability produced by a single pump photon to be ${10}^{\ensuremath{-}5}$, which is a significant improvement from the state of the art, and the photon-photon coupling strength to be 9.1 MHz. Our results mark steady progress toward quantum nonlinear optics at the ultimate single-photon limit, with potential applications in highly integrated photonics and quantum optical computing.

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