Photoluminescence Enhancement Dependent on the Orientations of Single NV Centers in Nanodiamonds on a Gold Film

Abstract

We studied the orientations of single Nitrogen-Vacancy (NV) color centers in nanodiamonds on a gold film by defocused imaging with a scanning confocal microscopy system and an electron-multiplying charge-coupled device. It was demonstrated that the perpendicular oriented dipole of single NV color center showed shorter fluorescence lifetime and higher fluorescence intensity than any other oriented ones on account of higher coupling efficiency of local electronic field induced by the surface plasmon resonance on the gold film for a vertical transition dipole.