Abstract
Photodissociation of H2S has been studied at 193.3 nm using H atom photofragment-translational spectroscopy with mass-spectrometric detection. H + HS(v) product branching ratios are reported which are not in quantitative agreement with other recent experimental results. Secondary photodissociation of HS radicals has also been observed, showing that both S(3P) and S(1D) are produced via perpendicular transition. The HS bond energy was found to be 3.62 ± 0.03 eV.
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