Abstract
The photocatalytic reduction of CO2 and H2O with triethylamine occurred using a cobalt(ii) chlorin complex adsorbed on multi-walled carbon nanotubes as a catalyst to yield CO and H2 with a high turnover number of 710.
Highlights
Photocatalytic reduction of CO2 and H2O to carbon monoxide (CO) and H2 with a cobalt chlorin complex adsorbed on multi-walled carbon nanotubes†
The photocatalytic reduction of CO2 and H2O with triethylamine occurred efficiently using a cobaltIJII) chlorin complex adsorbed on multi-walled carbon nanotubes as a CO2 reduction catalyst and [RuIIIJMe2phen)3]2+ (Me2phen = 4,7-dimethyl-1,10-phenanthroline) as a photocatalyst to yield CO and H2 with a ratio of 2.4 : 1 and a high turnover number of 710
Photocatalytic reduction of carbon dioxide (CO2) and water (H2O) to produce synthesis gas, which is a fuel gas mixture consisting primarily of hydrogen (H2) and carbon monoxide (CO), has merited significant interest, because synthetic gas can be converted to liquid hydrocarbon fuels by Fischer– Tropsch processes.[1,2,3,4,5,6]
Summary
Photocatalytic reduction of CO2 and H2O to CO and H2 with a cobalt chlorin complex adsorbed on multi-walled carbon nanotubes†. The photocatalytic reduction of CO2 and H2O with triethylamine occurred efficiently using a cobaltIJII) chlorin complex adsorbed on multi-walled carbon nanotubes as a CO2 reduction catalyst and [RuIIIJMe2phen)3]2+ (Me2phen = 4,7-dimethyl-1,10-phenanthroline) as a photocatalyst to yield CO and H2 with a ratio of 2.4 : 1 and a high turnover number of 710.
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