Abstract

Mesoporous SiO2 templates deposited TiO2 nanocrystals are synthesized via a sol–gel route, and Au nanoparticles (NPs) are deposited in the tubular mesopores of the templates by a photodeposition method (Au/SiO2–TiO2). The photocatalytic characteristics of Au/SiO2–TiO2 are discussed with the action spectra of photoreactions of 2-propanol and methylene blue. Photocatalytic activities of SiO2–TiO2 under individual ultraviolet (UV) and visible (Vis) light illumination are enhanced by deposition of Au NPs. Furthermore, Au/SiO2–TiO2 shows higher photocatalytic activities under simultaneous irradiation of UV and Vis light compared to the activity under individual UV and Vis light irradiation. Since the photocatalytic activity under simultaneous irradiation is almost the same as the total activities under individual UV and Vis light irradiation, it is concluded that the electrons and the holes generated by lights of different wavelengths are efficiently used for photocatalysis without carrier recombination.

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