Abstract
H2O2 was produced from H2O and O2 using cyano-bridged polynuclear transition metal complexes as water oxidation catalysts with a Ru photocatalyst in water under visible light irradiation.
Highlights
Photocatalytic production of hydrogen peroxide from water and dioxygen using cyano-bridged polynuclear transition metal complexes as water oxidation catalysts†
Hydrogen peroxide was produced efficiently from water and dioxygen using [RuIIIJMe2phen)3]2+ (Me2phen = 4,7-dimethyl-1,10phenanthroline) as a photocatalyst and cyano-bridged polynuclear transition metal complexes composed of Fe and Co as water oxidation catalysts in the presence of Sc3+ in water under visible light irradiation
It is highly desired to improve the catalytic activity for the photocatalytic production of H2O2 from H2O2 production from water (H2O) and O2 (ΔG° = 210 kJ mol−1, eqn (1)) using earth-abundant metal catalysts.[15,16,17]
Summary
Photocatalytic production of hydrogen peroxide from water and dioxygen using cyano-bridged polynuclear transition metal complexes as water oxidation catalysts†. Hydrogen peroxide was produced efficiently from water and dioxygen using [RuIIIJMe2phen)3]2+ (Me2phen = 4,7-dimethyl-1,10phenanthroline) as a photocatalyst and cyano-bridged polynuclear transition metal complexes composed of Fe and Co as water oxidation catalysts in the presence of Sc3+ in water under visible light irradiation.
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