Phenomenological model of the magnetocaloric effect and its correlation with critical behavior near room temperature in La0.7Ca0.2Sr0.1MnO3 manganite

Abstract

In this paper, we investigate the field dependence of the magnetocaloric properties of La0.7Ca0.2Sr0.1MnO3 powder sample using a phenomenological model. Our compound was elaborated by the conventional solid state reaction. The model parameters were determined from the magnetization data and were used to give better fits to magnetic transition and to calculate the magnetocaloric quantities. The magnetocaloric parameters such as the maximum of the magnetic entropy change \(\Delta S_M^{max}\) and the relative cooling power RCP, have been determined from the calculation of the magnetization as a function of temperature under several magnetic applied field. Thus, from the magnetocaloric results, such as RCP ≈ b(μ0H)1+1/δ and Tpeak − TC ≈ b (µ0H)1/Δ, the critical exponents values related to the magnetic transition have been determined. The estimated results are close to those expected by the tricritical mean-field model. Furthermore, the values of the ferromagnetic transition temperature TC, as well as the critical exponents β, γ and δ obtained by the theoretical model, are compared with those obtained by other various techniques (such as the modified Arrott plots, the Kouvel–Fisher method and the critical isotherm analysis). A good agreement has been found in the vicinity of the Curie temperature.