Perovskite/Organic Semiconductor-Based Photonic Synaptic Transistor for Artificial Visual System.

Abstract

Artificial visual system with information sensing, processing, and memory function is promoting the development of artificial intelligence techniques. Photonic synapse as an essential component can enhance the visual information processing efficiency owing to the high propagation speed, low latency, and large bandwidth. Herein, photonic synaptic transistors based on organic semiconductor poly[2,5-(2-octyldodecyl)-3,6-diketopyrrolopyrrole-alt-5,5-(2,5-di(thien-2-yl)thieno [3,2-b]thiophene)] (DPPDTT) and perovskite CsPbBr3 quantum dots are fabricated by a simple solution process. The device can simulate fundamental synaptic behaviors, including excitatory postsynaptic current, pair-pulse facilitation, the transition of short-term memory to long-term memory, and "learning experience" behavior. Combining the advantages of the high photosensitivity of perovskites and relatively high conductivity of DPPDTT, the device can exhibit excellent synaptic performances at a low voltage of -0.2 V. Even under an ultralow operation voltage of -0.0005 V, the device can still show obvious synaptic responses. Tunable synaptic integration behaviors including "AND" and "OR" light logic functions can be realized. An artificial visual system is successfully emulated by illuminating the synaptic arrays employing light of different densities. Therefore, low-voltage synaptic devices based on organic semiconductor and CsPbBr3 quantum dots with a simple fabrication technique present high potential to mimic human visual memory.