Abstract
Understanding the fracture properties of graphene sheets is a crucial step towards their practical applications. However, due to the limitations of experimental operations and all-atom (AA) methods, investigating the fracture of large-sized nano graphene sheets remains a formidable challenge. Especially, study on the layer-by-layer fracture of multi-layer graphene sheets (MLGS) is nearly impossible. To overcome this challenge, a peridynamic (PD) model is proposed in this study, which comprises the intra-layer part and the inter-layer part. The proposed PD model is validated by comparing the fracture toughness and the fracture forms of MLGS with existing experiments. It is found that the uniaxial tensile stress-strain curve of pre-cracked MLGS is closely related to the number of graphene layers in MLGS. The fracture property of MLGS can be enhanced by increasing the number of graphene layers, reducing the pre-crack length and blunting the pre-crack tip. Notably, asynchronous crack propagation with independent path observed in MLGS is a unique mechanism for strengthening the fracture property, which is distinct from monolayer graphene sheet. In this work, the PD theory is extended for the first time to investigate the in-plane fracture of large-sized nano MLGS.
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