Abstract

Structuring metal surfaces on the nanoscale has been shown to alter their fundamental processes like reflection or absorption by supporting surface plasmon resonances. Here, we propose metal films with subwavelength rectangular nanostructuring that perfectly absorb the incident radiation in the optical regime. The structures are fabricated with low-cost nanoimprint lithography and thus constitute an appealing alternative to elaborate absorber designs with complex meta-atoms or multilayer structuring. We conduct a thorough numerical analysis to gain physical insight on how the key structural parameters affect the optical response and identify the designs leading to broad spectral and angular bandwidths, both of which are highly desirable in practical absorber applications. Subsequently, we fabricate and measure the structures with an FT-IR spectrometer demonstrating very good agreement with theory. Finally, we assess the performance of the proposed structures as sensing devices by quantifying the dependence of the absorption peak frequency position on the superstrate material.

Highlights

  • Surface plasmon polaritons (SPPs) are electromagnetic surfaces waves coupled to free electron oscillations [1,2,3,4]

  • We have investigated how the key structural parameters (a, h, s) affect the optical response of our nanostructured metal film

  • Typical silicon (Si) master molds were realized by electron beam lithography and reactive ion etching steps

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Summary

Introduction

Surface plasmon polaritons (SPPs) are electromagnetic surfaces waves coupled to free electron oscillations [1,2,3,4]. Besides efficient coupling to propagating SPPs [5,6,7], metallic gratings can be used as Bragg reflectors to route propagating signals in guided wave circuits [8,9,10,11] or form wavelength-selective components [12,13,14] They can serve as diffractive optical elements deflecting free-space beams to the desired direction [15,16]. Another prominent example is planar, uniform multi-layer structures comprising lossy dielectric and metal layers [29,30] In these cases, it becomes necessary to process different materials for covering different frequencies of operation [30].

Geometric and material parameters
Optical response: perfect absorption in the visible regime
Experimental verification of perfect optical absorption
Findings
Conclusions
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