Abstract
Vibrational spectra of TlInS2 crystals in the terahertz frequency range (0.1–3 THz) have been obtained and analyzed. The observed low-frequency band is attributed to the libration oscillations of nanolayers (so-called boson peak). A correlation between the coherent low-frequency oscillation and a disordered character of the crystal structure is shown. A conclusion is made on the presence of a topological disorder that manifests itself on the layered subsystem level.
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